Something's not "right" in this deal, from what I've read . . .
There are basically two sizes of C-body radiators, width-wise. The '66 and back had the round top, newer ones had the square top tank, but still the same width and size. So, how was it determined that you got the "correct size"? Dimensions or otherwise?
The cars came with a 180 degree thermostat. The 195 degree thermostat came in the later 1960s, but in '72, it was a 185 degree OEM thermostat. NO significant differences in how "hot" they ran due to this.
What type of fan? Direct drive, thermal, flex fan, size, number of blades? My theory is that the thermal clutch 7-blade fan is best. A flex fan might be lighter, but might block air flow through the radiator at higher fan rpms, as it feathers-out. Fan shroud should match and is needed.
Getting all of the air through the radiator is important, which is why Chrysler had their "yoke seal" on the bottom of the hood, to go between the radiator tank and the top of the core support when the hood is closed. Decreasing gaps between the side of the radiator might help too, but Chryslers were not nearly as bad as GMs were about gaps on the sides of the radiators.
Hopefully, the water pump pulley is the correct one to have the correct drive ratio for the water pump and a/c or non-a/c water pump. The a/c pump has fewer vanes, but it runs about 40% faster due to the different drive ratio. "Drive ratio" is in comparison to the crankshaft pulley size.
I've run my '66 Newport 383 a/c car with a defective vacuum advance and all it did was to consume more gas. No overheating issue due to the "retarded" spark as it was on only mechanical advance when the vacuum adv wasn't working. It would take a very lean mixture to result in overheating, although many diagnostic lists mention carb mixture as a "cause". IF it's THAT lean, you'll know by how it's NOT running well. The original Lean Burns were spec'd for a 16:1 mixture, rather than the normal 14.7:1, with no larger radiators or other changes to the cooling system.
Using the heat gun, what are the temps you're finding? At the thermostat, at the water pump, at the radiator top core, and at the radiator bottom of the core? Even with the OEM parts, Chrysler C-body cars (and others) usually did NOT have any overheat problems when new. Much less than Fords and GMs back then. That has been my observations over the years . . . unless something's mechanically wrong. Bad fan clutch, internally restricted radiator core, lower hose issues, etc. What engine, rear axle, tire size combination?
To me, stay away from the "high flow" noted items. As noted, there is an optimum speed of the coolant through the block for best heat transfer. Other than the water pump, that flow is regulated by the restrictions in the head gaskets. If the gaskets are original and the coolant hasn't been serviced as it should have been, flow over the many miles and poor maintenance can erode these hole and enlarge them. An outside chance, but I don't know that THAT would cause overheating.
Too much new stuff with no improvement. Doesn't all add up.
CBODY67